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窪田 崇秀*; 高野 大地*; 小田 洋平*; Mohanty, S.*; 伊藤 啓太*; 松木 充弘*; 林田 誠弘*; Sun, M.*; 竹田 幸治; 斎藤 祐児; et al.
Physical Review Materials (Internet), 6(4), p.044405_1 - 044405_12, 2022/04
被引用回数:5 パーセンタイル:56.94(Materials Science, Multidisciplinary)This study focuses on an inverse-type Heusler alloy, MnCoGa (MCG), with a small off-stoichiometry (), showing perpendicular magnetic anisotropy (PMA). We observed a relatively large uniaxial magnetocrystalline anisotropy constant () on the order of 10 J/m at room temperature in the MCG films with a small tetragonal distortion of a few percent. X-ray magnetic circular dichroism (XMCD) was employed to get insight into the origin for the PMA. Negligible angular variation of the orbital magnetic moment evaluated using the XMCD spectra suggested a minor role of the so-called Bruno's term to . The origin of the PMA was discussed based on the second-order perturbation theory in terms of the spin-orbit coupling, and first principles calculations, claiming that the mixing of the occupied - and the unoccupied -spin states is responsible for the PMA of the MCG films.
河野 嵩*; 鹿子木 将明*; 吉川 智己*; Wang, X.*; 角田 一樹*; 宮本 幸治*; 室 隆桂之*; 竹田 幸治; 斎藤 祐児; 後藤 一希*; et al.
Physical Review B, 100(16), p.165120_1 - 165120_6, 2019/10
被引用回数:5 パーセンタイル:27.17(Materials Science, Multidisciplinary)Resonant photoelectron spectroscopy at the Co and Mn 2 core absorption edges of half-metallic CoMnGe has been performed to determine the element-specific density of states (DOS). A significant contribution of the Mn 3 partial DOS near the Fermi level () was clarified by measurement at the Mn 2 absorption edge. Further analysis by first-principles calculation revealed that it has symmetry, which must be responsible for the electrical conductivity along the line perpendicular to the film plane. The dominant normal Auger contribution observed at the Co 2 absorption edge indicates delocalization of photoexcited Co 3 electrons. The difference in the degrees of localization of the Mn 3 and Co 3 electrons in CoMnGe is explained by the first-principles calculation.
土屋 朋生*; 小林 亮太*; 窪田 崇秀*; 斉藤 耕太郎*; 小野 寛太*; 大原 高志; 中尾 朗子*; 高梨 弘毅*
Journal of Physics D; Applied Physics, 51(6), p.065001_1 - 065001_7, 2018/02
被引用回数:10 パーセンタイル:45.49(Physics, Applied)MnVAl Heusler alloy films were epitaxially grown on MgO(100) single-crystal substrates by ultra-high-vacuum magnetron sputtering. A2- and L21-type MnVAl order was controlled by the deposition temperature. A2-type MnVAl films showed no spontaneous magnetization, while L21-type MnVAl films showed ferrimagnetic behaviour with a maximum saturation magnetization of 220 emu/cm at room temperature (RT). An antiferromagnetic reflection was observed with neutron diffraction at RT for an A2-type MnVAl film deposited at 400C. A bilayer sample of the antiferromagnetic A2-type MnVAl and Fe showed an exchange bias of 120 Oe at 10 K.
藤原 秀紀*; 向後 純也*; 笠原 理加*; 西岡 拓真*; 藤本 直央*; 永井 浩大*; 関山 明*; 角田 一樹; 竹田 幸治; 斎藤 祐児; et al.
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ホイスラー合金の磁気特性や電子構造は、結晶の化学量論的不安定性や結晶構造の長距離規則度に大きく依存することが広く知られている。本研究では、結晶構造の規則度と磁気特性の相関を明らかにするため、CoMnSi純良単結晶試料に対し、広域X線吸収微細構造(EXAFS)の磁気円二色性をSPring-8のBL23SUにおいて測定した。そして、EXAFS振動とは周期の異なる明瞭な磁気EXAFS振動を見出した。この結果は、多重散乱理論に基づく解析により、遠方磁性サイトの寄与が強く反映していることで説明できることを明らかにした。